Welcome to visit The Chinese Journal of Process Engineering, Today is
Process & Technology

Formation and characteristics of used activated coke from flue gas purification process by activated coke in moving bed

  • Fengqin YU Yunjia LI Zhouen LIU Wensong LI Weidong ZHANG Shiqiu GAO Guangwen XU Jian YU
Expand
  • 1. School of Chemical Engineering, Xiangtan University, Xiangtan, Hunan 411105, China 2. State Key Laboratory of Multi-phase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China 3. Jiangsu New Zhongjin Environmental Protection Technology Co., LTD., Yixing, Jiangsu 214200, China 4. Institute of Industrial Chemistry and Energy Technology, Shenyang University of Chemical Technology, Shenyang, Liaoning 110142, China

Received date: 2019-08-03

  Revised date: 2019-10-15

  Online published: 2020-06-19

Supported by

National Natural Science Foundation of China General Projects

Abstract

The multi-pollutant removal using activated coke (AC) in moving bed under low temperature and dry state showed great prospect in desulfurization and denitrification process of flue gas from steel sintering process. The abrasion of AC in this process was the crucial factors which restricted the wide application of this technology. Being aimed at the used AC which was produced in the process of SOx and NOx removal from Baogang sintering flue gas, the texture properties, including the specific surface area, pore volume structure, the content of heavy metals and alkali metals in ash, surface functional group characteristics and desulfurization and denitration performance of AC were investigated to obtain the formation and variation behavior of used AC. Compared to fresh AC, an obvious increase in the content of N, S and O elements and transition metal oxides were observed in the used AC powder in particle size at 0.2?5 mm, and its specific surface area also increased from 191.0 m2/g to 499.0 m2/g. As a result, the NO conversion rate increased greatly from 20% to 70% at 150℃, and the penetrating sulfur capacity was enhanced from 0.27 mg SO2/g to 11.08 mg SO2/g at 120℃. The used AC exhibited a good potentiality for reutilization.

Cite this article

Fengqin YU Yunjia LI Zhouen LIU Wensong LI Weidong ZHANG Shiqiu GAO Guangwen XU Jian YU . Formation and characteristics of used activated coke from flue gas purification process by activated coke in moving bed[J]. The Chinese Journal of Process Engineering, 2020 , 20(6) : 695 -702 . DOI: 10.12034/j.issn.1009-606X.219268

Outlines

/